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Synthetic studies toward FR182877. Remarkable solvent effect in the vinylogous morita-baylis-hillman cyclization

Academic Article
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Overview

authors

  • Methot, J. L.
  • Roush, William

publication date

  • October 2003

journal

  • Organic Letters  Journal

abstract

  • [reaction: see text]. The intramolecular vinylogous Morita-Baylis-Hillman reaction was explored to access the central cyclopentane ring of FR182877. The reaction manifold and product distribution is strikingly solvent and substrate dependent.

subject areas

  • Catalysis
  • Cyclization
  • Molecular Conformation
  • Molecular Structure
  • Organotin Compounds
  • Phosphines
  • Polycyclic Compounds
  • Solvents
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Identity

International Standard Serial Number (ISSN)

  • 1523-7060

Digital Object Identifier (DOI)

  • 10.1021/ol0357550

PubMed ID

  • 14572290
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Additional Document Info

start page

  • 4223

end page

  • 4226

volume

  • 5

issue

  • 22

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