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Ligand-enabled meta-C-H alkylation and arylation using a modified norbornene

Academic Article
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Overview

related to degree

  • Shen, Pengxiang, Ph.D. in Chemistry, Scripps Research 2014 - 2019
  • Zhu, Ru-Yi, Ph.D. in Chemistry, Scripps Research 2013 - 2018

authors

  • Shen, Pengxiang
  • Wang, X. C.
  • Wang, P.
  • Zhu, Ru-Yi
  • Yu, Jin-Quan

publication date

  • September 2015

journal

  • Journal of the American Chemical Society  Journal

abstract

  • 2-Carbomethoxynorbornene is identified as a more effective transient mediator to promote a Pd(II)-catalyzed meta-C(sp(2))-H alkylation of amides with various alkyl iodides as well as arylation with previously incompatible aryl iodides. The use of a tailor-made quinoline ligand is also crucial for this reaction to proceed.

subject areas

  • Alkylation
  • Hydrocarbons, Cyclic
  • Ligands
  • Norbornanes
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Identity

PubMed Central ID

  • PMC4573956

International Standard Serial Number (ISSN)

  • 0002-7863

Digital Object Identifier (DOI)

  • 10.1021/jacs.5b08914

PubMed ID

  • 26313012
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Additional Document Info

start page

  • 11574

end page

  • 11577

volume

  • 137

issue

  • 36

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