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Sarlah, David

Graduate Student

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Positions

• 2014 - Faculty Member, University of Illinois at Urbana-Champaign

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• Doctoral Dissertation

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Publications

recent publications

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  • Hernandez, L. W., Sarlah, D. Empowering synthesis of complex natural products Chemistry-a European Journal  2019  DOI:10.1002/chem.201901808  PMID:31194262
  • Tang, C., Okumura, M., Zhu, Y., Hooper, A. R., Zhou, Y., Lee, Y. H., Sarlah, D. Palladium-catalyzed dearomative syn-1,4-carboamination with Grignard reagents Angewandte Chemie-International Edition  2019 58:10245-10249  DOI:10.1002/anie.201905021  PMID:31090252  PMCID:PMC6640109
  • Dennis, D. G., Okumura, M., Sarlah, D. Synthesis of (+/-)-idarubicinone via global functionalization of tetracene Journal of the American Chemical Society  2019 141:10193-10198  DOI:10.1021/jacs.9b05370  PMID:31244190
  • Bingham, T. W., Hernandez, L. W., Olson, D. G., Svec, R. L., Hergenrother, P. J., Sarlah, D. Enantioselective synthesis of isocarbostyril alkaloids and analogs using catalytic dearomative functionalization of benzene Journal of the American Chemical Society  2019 141:657-670  DOI:10.1021/jacs.8b12123  PMID:30520639  PMCID:PMC6488038
  • Wertjes, W. C., Okumura, M., Sarlah, D. Palladium-catalyzed dearomative syn-1,4-diamination Journal of the American Chemical Society  2019 141:163-167  DOI:10.1021/jacs.8b13030  PMID:30566338  PMCID:PMC6488036
  • Wertjes, W. C., Southgate, E. H., Sarlah, D. Recent advances in chemical dearomatization of nonactivated arenes Chemical Society Reviews  2018 47:7996-8017  DOI:10.1039/c8cs00389k  PMID:30073226
  • Hernandez, L. W., Klockner, U., Pospech, J., Hauss, L., Sarlah, D. Nickel-catalyzed dearomative trans-1,2-carboamination Journal of the American Chemical Society  2018 140:4503-4507  DOI:10.1021/jacs.8b01726  PMID:29544244  PMCID:PMC5971658
  • Okumura, M., Sarlah, D. Arenophile-mediated dearomative functionalization strategies Synlett  2018 29:845-855  DOI:10.1055/s-0036-1591940
  • Sarlah, D., Okumura, M., Shved, A. Palladium-catalyzed dearomative syn-1,4-carboamination Synlett  2018 29:A40-A43
  • Sarlah, D., Okumura, M., Shved, A. Palladium-catalyzed dearomative syn-1,4-carboamination Synthesis-Stuttgart  2018 50:A40-A43  DOI:10.1055/s-0036-1591457  PMID:29183109  PMCID:PMC5971112
  • Okumura, M., Shved, A. S., Sarlah, D. Palladium-catalyzed dearomative syn-1,4-carboamination Journal of the American Chemical Society  2017 139:17787-17790  DOI:10.1021/jacs.8b13030  PMID:29183109  PMCID:PMC5971112
  • Hernandez, L. W., Pospech, J., Klockner, U., Bingham, T. W., Sarlah, D. Synthesis of (+)-pancratistatins via catalytic desymmetrization of benzene Journal of the American Chemical Society  2017 139:15656-15659  DOI:10.1021/jacs.7b10351  PMID:29059521  PMCID:PMC5960067
  • Schafroth, M. A., Rummelt, S. M., Sarlah, D., Carreira, E. M. Enantioselective iridium-catalyzed allylic cyclizations Organic Letters  2017 19:3235-3238  DOI:10.1021/acs.orglett.7b01346  PMID:28573860
  • Southgate, E. H., Holycross, D. R., Sarlah, D. Total synthesis of lycoricidine and narciclasine by chemical dearomatization of bromobenzene Angewandte Chemie-International Edition  2017 56:15049-15052  DOI:10.1002/anie.201709712  PMID:29024240  PMCID:PMC5971115
  • Okumura, M., Huynh, S. M. N., Pospech, J., Sarlah, D. Arenophile-mediated dearomative reduction Angewandte Chemie-International Edition  2016 55:15910-15914  DOI:10.1002/anie.201609686  PMID:27879027  PMCID:PMC6043355
  • Southgate, E. H., Pospech, J., Fu, J., Holycross, D. R., Sarlah, D. Dearomative dihydroxylation with arenophiles Nature Chemistry  2016 8:922-928  DOI:10.1038/nchem.2594  PMID:27657867  PMCID:PMC5971114
  • Sarlah, D. Organic chemistry: No double bond left behind Nature  2016 531:453-454  PMID:27008963
  • Sarlah, D., Juranovic, A., Kozar, B., Rejc, L., Golobic, A., Petric, A. Synthesis of naphthalene-based push-pull molecules with a heteroaromatic electron acceptor Molecules  2016 21  DOI:10.3390/molecules21030267  PMID:26950099
  • Ungarean, C. N., Southgate, E. H., Sarlah, D. Enantioselective polyene cyclizations Organic & Biomolecular Chemistry  2016 14:5454-5467  DOI:10.1039/c6ob00375c  PMID:27143099
  • Hamilton, J. Y., Sarlah, D., Carreira, E. M. Iridium-catalyzed enantioselective allylic alkylation with functionalized organozinc bromides Angewandte Chemie-International Edition  2015 54:7644-7647  DOI:10.1002/anie.201501851  PMID:25969352
  • Shemet, A., Sarlah, D., Carreira, E. M. Stereochemical studies of the opening of chloro vinyl epoxides: cyclic chloronium ions as intermediates Organic Letters  2015 17:1878-1881  DOI:10.1021/acs.orglett.5b00558  PMID:25811099
  • Schafroth, M. A., Zuccarello, G., Krautwald, S., Sarlah, D., Carreira, E. M. Stereodivergent total synthesis of Δ9-tetrahydrocannabinols Angewandte Chemie - International Edition  2014 53:13898-13901  DOI:10.1002/anie.201408380  PMID:25303495
  • Hamilton, J. Y., Hauser, N., Sarlah, D., Carreira, E. M. Iridium-catalyzed enantioselective allyl-allylsilane cross-coupling Angewandte Chemie - International Edition  2014 53:10759-10762  DOI:10.1002/anie.201406077  PMID:25111443
  • Hamilton, J. Y., Sarlah, D., Carreira, E. M. Iridium-catalyzed enantioselective allyl-alkene coupling Journal of the American Chemical Society  2014 136:3006-3009  DOI:10.1021/ja412962w  PMID:24521052
  • Krautwald, S., Schafroth, M. A., Sarlah, D., Carreira, E. M. Stereodivergent α-allylation of linear aldehydes with dual iridium and amine catalysis Journal of the American Chemical Society  2014 136:3020-3023  DOI:10.1021/ja5003247  PMID:24506196
  • Lin, T. Y., Chin, C. R., Everitt, A. R., Clare, S., Perreira, J. M., Savidis, G., Aker, A. M., John, S. P., Sarlah, D., Carreira, E. M., Elledge, S. J., Kellam, P., et al. Amphotericin B increases influenza A virus infection by preventing IFITM3-mediated restriction Cell Reports  2013 5:895-908  DOI:10.1016/j.celrep.2013.10.033  PMID:24268777  PMCID:PMC3898084
  • Hamilton, J. Y., Sarlah, D., Carreira, E. M. Iridium-catalyzed enantioselective allylic alkynylation Angewandte Chemie - International Edition  2013 52:7532-7535  DOI:10.1002/anie.201302731  PMID:23712914
  • Krautwald, S., Sarlah, D., Schafroth, M. A., Carreira, E. M. Enantio- and diastereodivergent dual catalysis: α-allylation of branched aldehydes Science  2013 340:1065-1068  DOI:10.1126/science.1237068  PMID:23723229
  • Hamilton, J. Y., Sarlah, D., Carreira, E. M. Iridium-catalyzed enantioselective allylic vinylation Journal of the American Chemical Society  2013 135:994-997  DOI:10.1021/ja311422z  PMID:23256708
  • Schafroth, M. A., Sarlah, D., Krautwald, S., Carreira, E. M. Iridium-catalyzed enantioselective polyene cyclization Journal of the American Chemical Society  2012 134:20276-20278  DOI:10.1021/ja310386m  PMID:23193947
  • Nicolaou, K. C., Lu, M., Totokotsopoulos, S., Heretsch, P., Giguere, D., Sun, Y. P., Sarlah, D., Nguyen, T. H., Wolf, I. C., Smee, D. F., Day, C. W., Bopp, S., et al. Synthesis and biological evaluation of epidithio-, epitetrathio-, and bis-(methylthio)diketopiperazines: synthetic methodology, enantioselective total synthesis of epicoccin G, 8,8'-epi-ent-rostratin B, gliotoxin, gliotoxin G, emethallicin E, and haematocin and discovery of new antiviral and antimalarial agents Journal of the American Chemical Society  2012 134:17320-17332  DOI:10.1021/ja308429f  PMID:22978674  PMCID:PMC3490634
  • Nicolaou, K. C., Sun, Y. P., Sarlah, D., Zhan, W. Q., Wu, T. R. Bioinspired synthesis of hirsutellones A, B, and C Organic Letters  2011 13:5708-5710  DOI:10.1021/ol202239u  PMID:21913732  PMCID:PMC3207260
  • Nicolaou, K. C., Totokotsopoulos, S., Giguere, D., Sun, Y. P., Sarlah, D. Total synthesis of epicoccin G Journal of the American Chemical Society  2011 133:8150-8153  DOI:10.1021/ja2032635  PMID:21548595  PMCID:PMC3102137
  • Nicolaou, K. C., Sanchini, S., Sarlah, D., Lu, G., Wu, T. R., Nomura, D. K., Cravatt, B. F., Cubitt, B., de la Torre, J. C., Hessell, A. J., Burton, D. R. Design, synthesis, and biological evaluation of a biyouyanagin compound library Proceedings of the National Academy of Sciences of the United States of America  2011 108:6715-6720  DOI:10.1073/pnas.1015258108  PMID:21245351  PMCID:PMC3084107
  • Nicolaou, K. C., Sun, Y. P., Korman, H., Sarlah, D. Asymmetric total synthesis of cylindrocyclophanes A and F through cyclodimerization and a Ramberg-Bäcklund reaction Angewandte Chemie-International Edition  2010 49:5875-5878  DOI:10.1002/anie.201003500  PMID:20623817  PMCID:PMC3014728
  • Nicolaou, K. C., Sanchini, S., Wu, T. R., Sarlah, D. Total synthesis and structural revision of biyouyanagin B Chemistry-a European Journal  2010 16:7678-7682  DOI:10.1002/chem.201001474  PMID:20572192  PMCID:PMC3023179
  • Nicolaou, K. C., Reingruber, R., Sarlah, D., Brase, S. Enantioselective intramolecular Friedel−Crafts-type α-arylation of aldehydes Journal of the American Chemical Society  2009 131:2086-2087  DOI:10.1021/ja809405c  PMID:19173649
  • Nicolaou, K. C.*, Sarlah, D.*, Wu, T. R., Zhan, W. Q. Total synthesis of hirsutellone B Angewandte Chemie-International Edition  2009 48:6870-6874  DOI:10.1002/anie.200903382  PMID:19685548  PMCID:PMC2772144 (* = equal contribution)
  • Nicolaou, K. C., Wu, T. R., Sarlah, D., Shaw, D. M., Rowcliffe, E., Burton, D. R. Total synthesis, revised structure, and biological evaluation of biyouyanagin A and analogues thereof Journal of the American Chemical Society  2008 130:11114-11121  DOI:10.1021/ja802805c  PMID:18646750  PMCID:PMC2614900
  • Dai, M., Sarlah, D., Yu, M., Danishefsky, S. J., Jones, G. O., Houk, K. N. Highly selective Diels-Alder reactions of directly connected enyne dienophiles Journal of the American Chemical Society  2007 129:645-657  DOI:10.1021/ja065762u  PMID:17227028
  • Nicolaou, K. C.*, Sarlah, D.*, Shaw, D. M. Total synthesis and revised structure of biyouyanagin A Angewandte Chemie-International Edition  2007 46:4708-4711  DOI:10.1002/anie.200701552  PMID:17523208 (* = equal contribution)
  • Nicolaou, K. C., Pihko, P. M., Bernal, F., Frederick, M. O., Qian, W. Y., Uesaka, N., Diedrichs, N., Hinrichs, J., Koftis, T. V., Loizidou, E., Petrovic, G., Rodriquez, M., et al. Total synthesis and structural elucidation of azaspiracid-1. Construction of key building blocks for originally proposed structure Journal of the American Chemical Society  2006 128:2244-2257  DOI:10.1021/ja0547477  PMID:16478178
  • Zorko, M., Majerle, A., Sarlah, D., Keber, M. M., Mohar, B., Jerala, R. Combination of antimicrobial and endotoxin-neutralizing activities of novel oleoylamines Antimicrobial Agents and Chemotherapy  2005 49:2307-2313  DOI:10.1128/;aac.49.6.2307-2313.2005  PMID:15917526  PMCID:PMC1140490
  • Nicolaou, K. C., Bulger, P. G., Sarlah, D. Metathesis reactions in total synthesis Angewandte Chemie-International Edition  2005 44:4490-4527  DOI:10.1002/anie.200500369  PMID:16003791
  • Nicolaou, K. C., Bulger, P. G., Sarlah, D. Palladium-catalyzed cross-coupling reactions in total synthesis Angewandte Chemie-International Edition  2005 44:4442-4489  DOI:10.1002/anie.200500368  PMID:15991198

Background

education and training

• Ph.D. in Chemistry, Scripps Research 2006 - 2011
• B.S. in Chemistry, University of Ljubljana 2006

advisee of

• graduate advising relationship

  • Nicolaou, K.C., Ph.D.  candidacy, 2007 - 2011

Contact

full name

• David Sarlah

geographic location

• Scripps California 

Identity

ORCID iD

• http://orcid.org/0000-0002-8736-8953

Scopus ID

• 16680405500